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High-Performance Flexible Asymmetric Supercapacitor Based on CoAl-LDH and rGO Electrodes
Nano-Micro Letters ( IF 26.6 ) Pub Date : 2017-02-18 , DOI: 10.1007/s40820-017-0134-8
Shuoshuo Li , Pengpeng Cheng , Jiaxian Luo , Dan Zhou , Weiming Xu , Jingwei Li , Ruchun Li , Dingsheng Yuan

A flexible asymmetric supercapacitor (ASC) based on a CoAl-layered double hydroxide (CoAl-LDH) electrode and a reduced graphene oxide (rGO) electrode was successfully fabricated. The CoAl-LDH electrode as a positive electrode was synthesized by directly growing CoAl-LDH nanosheet arrays on a carbon cloth (CC) through a facile hydrothermal method, and it delivered a specific capacitance of 616.9 F g−1 at a current density of 1 A g−1. The rGO electrode as a negative electrode was synthesized by coating rGO on the CC via a simple dip-coating method and revealed a specific capacitance of 110.0 F g−1 at a current density of 2 A g−1. Ultimately, the advanced ASC offered a broad voltage window (1.7 V) and exhibited a high superficial capacitance of 1.77 F cm−2 at 2 mA cm−2 and a high energy density of 0.71 mWh cm−2 at a power density of 17.05 mW cm−2, along with an excellent cycle stability (92.9% capacitance retention over 8000 charge–discharge cycles).

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中文翻译:

基于CoAl-LDH和rGO电极的高性能柔性不对称超级电容器

成功地制造了基于CoAl层状双氢氧化物(CoAl-LDH)电极和氧化石墨烯(rGO)电极的柔性不对称超级电容器(ASC)。通过简便的水热法在碳布(CC)上直接生长CoAl-LDH纳米片阵列,合成了作为正极的CoAl-LDH电极,并在电流密度为1的情况下提供了616.9 F g -1的比电容。A g -1。通过使用简单的浸涂法在CC上涂覆rGO来合成作为负极的rGO电极,并在2 A g -1的电流密度下显示出110.0 F g -1的比电容。。最终,先进的ASC提供了宽电压范围(1.7 V),并在2 mA cm -2下表现出1.77 F cm -2的高表面电容,在17.05 mW的功率密度下表现出0.71 mWh cm -2的高能量密度。cm -2,以及出色的循环稳定性(8000个充放电循环中92.9%的电容保持率)。

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更新日期:2017-02-18
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